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11.
RE2Si2O7 is one of the final products of the chemical interaction of radioactive cation simulators and the silicates used in the engineered barrier of deep geological repositories. The aim of this paper is to study the chemical and structural behaviour of Lu2Si2O7 (Lu as actinide tripositive state simulator) in several different chemical systems. The conditions expected at the repositories are simulated in the laboratory with solutions of different compositions and pH. Both the solid products and remnant solutions were analyzed using techniques that give information on the short- and long-range structural order. The results show good stability of Lu2Si2O7, under the studied conditions, and, therefore, encapsulation of the radioactive actinide cations as a disilicate phase could be considered a viable method to ensure the long-term safety of the repositories. 相似文献
12.
Janot Noémie Groenenberg Jan E. Otero-Fariña Alba Pinheiro José Paulo 《Aquatic Geochemistry》2021,27(2):127-140
Aquatic Geochemistry - The aim of this study was to develop an analytical method to determine free concentrations of Europium (Eu(III)) in natural waters. Europium(III) in solution was detected... 相似文献
13.
de Souza Luciana Sandra Bastos Silva Maiara Tatiane Lima Alba Elisiane de Moura Magna Soelma Beserra da Cruz Neto José Francisco de Souza Carlos André Alves da Silva Thieres George Freire 《Theoretical and Applied Climatology》2022,149(1-2):593-602
Theoretical and Applied Climatology - Analysing alternative methods for estimating reference evapotranspiration (ET0) is essential for improving the management of water resources, especially where... 相似文献
14.
Marc Peipoch Esperança Gacia Alba Blesa Miquel Ribot Joan L. Riera Eugènia Martí 《Aquatic Sciences - Research Across Boundaries》2014,76(2):203-215
We examined the relevance of dissolved inorganic nitrogen (DIN) forms (nitrate and ammonium) in stream water as N sources for different macrophyte species. To do this, we investigated the variability and relationships between 15N natural abundance of DIN forms and of four different macrophyte species in five different streams influenced by inputs from wastewater treatment plants and over time within one of these streams. Results showed that 15N signatures were similar in species of submersed and amphibious macrophytes and in stream water DIN, whereas 15N signatures of the riparian species were not. 15N signatures of macrophytes were generally closer to 15N signatures of nitrate, regardless of the species considered. Our results showed significant relationships between 15N signatures of DIN and those of submersed Callitriche stagnalis and amphibious Veronica beccabunga and Apium nodiflorum, suggesting stream water DIN as a relevant N source for these two functional groups. Moreover, results from a mixing model suggested that stream water DIN taken up by the submersed and amphibious species was mostly in the form of nitrate. Together, these results suggest different contribution to in-stream N uptake among the spatially-segregated species of macrophytes. While submersed and amphibious species can contribute to in-stream N uptake by assimilation of DIN, macrophyte species located at stream channel edges do not seem to rely on stream water DIN as an N source. Ultimately, these results add a functional dimension to the current use of macrophytes for the restoration of stream channel morphology, indicating that they can also contribute to reduce excess DIN in streams. 相似文献
15.
Sergio Archangelsky Viviana Barreda Mauro G. Passalia Maria Gandolfo Mercedes Prámparo Edgardo Romero Rubén Cúneo Alba Zamuner Ari Iglesias Magdalena Llorens Gabriela G. Puebla Mirta Quattrocchio Wolfgang Volkheimer 《Cretaceous Research》2009,30(5):1073-1082
In this report, we analyze the angiosperm fossil record (micro- and megafossil) from the central and southern basins of Argentina, southern South America, deposited between the late Barremian (128.3 Ma) to the end of the Coniacian (85.8 Ma). Based on this analysis, three major stages in the evolution of the angiosperms in the southernmost region of South America are established as follows: the late Barremian–Aptian, the latest Aptian-earliest Albian, and the middle Albian- Coniacian. The comparison between our fossil data set and those from Australia, North America, Asia and Europe suggest that the evolution and diversification of the angiosperms at mid and high latitudes in both hemispheres occurred roughly synchronously. 相似文献
16.
Alba Sanmiguel-Vallelado Juan I. López-Moreno Enrique Morán-Tejeda Esteban Alonso-González Francisco M. Navarro-Serrano Ibai Rico J. Julio Camarero 《水文研究》2020,34(10):2247-2262
Snowpacks and forests have complex interactions throughout the large range of altitudes where they co-occur. However, there are no reliable data on the spatial and temporal interactions of forests with snowpacks, such as those that occur in nearby areas that have different environmental conditions and those that occur during different snow seasons. This study monitored the interactions of forests with snowpacks in four forest stands in a single valley of the central Spanish Pyrenees during three consecutive snow seasons (2015/2016, 2016/2017 and 2017/2018). Daily snow depth data from time-lapse cameras were compared with snow data from field surveys that were performed every 10–15 days. These data thus provided information on the spatial and temporal changes of snow–water equivalent (SWE). The results indicated that forest had the same general effects on snowpack in each forest stand and during each snow season. On average, forest cover reduced the duration of snowpack by 17 days, reduced the cumulative SWE of the snowpack by about 60% and increased the spatial heterogeneity of snowpack by 190%. Overall, forest cover reduced SWE total accumulation by 40% and the rate of SWE accumulation by 25%. The forest-mediated reduction of the accumulation rate, in combination with the occasional forest-mediated enhancement of melting rate, explained the reduced duration of snowpacks beneath forest canopies. However, the magnitude and timing of certain forest effects on snowpack had significant spatial and temporal variations. This variability must be considered when selecting the location of an experimental site in a mountainous area, because the study site should be representative of surrounding areas. The same considerations apply when selecting a time period for study. 相似文献
17.
Land use/cover, landforms and fragmentation patterns in a tropical dry forest in the southern Pacific region of Mexico 总被引：1，自引：0，他引：1
Leopoldo Galicia Alba Esmeralda Zarco-Arista Karla Ivette Mendoza-Robles José Luis Palacio-Prieto Arturo García-Romero 《Singapore journal of tropical geography》2008,29(2):137-154
In spite of widely documented studies of deforestation rates and land use/cover changes in tropical dry forests in Mexico, relatively little is known about fragmentation patterns in such forests. This study defines the spatial distribution of landforms and land use/cover types the lower Papagayo River basin and examines their influence on fragmentation patterns and biological diversity in a tropical dry forest in that southern Pacific region. The land use/cover map was constructed from aerial photographs, Landsat TM imagery (2000) and fieldwork. Landform units were defined based on altitude, slope, lithology and morphology. Landscape fragmentation parameters were obtained using FRAGSTATS (version 3.3) considering the numbers of patches, mean, minimum and maximum patch size, edge density, total edge and connectivity. Results show tropical dry forest to be remnant vegetation (~11 per cent), characterized by isolation and low connectivity. Land use/cover types have different effects on fragmentation patterns. Agriculture and cattle raising produce similar numbers of patches, but with a different mean size; and human settlements have a scattered distribution pattern. The abandonment of rural agricultural livelihoods has favoured the expansion of secondary tropical dry forest characterized by continuity and high connectivity, which suggests a high regeneration potential from land abandonment. It can be concluded that tropical dry forest fragmentation and recovery at regional scales depend on such landscape attributes as lithology, slope, geomorphology and management. 相似文献
18.
This paper presents the results of a comprehensive investigation of the interaction of layered silicates with Ca(OH)2 in hydrothermal conditions. The study is intended to evaluate the stability of the clay buffer in radioactive waste repositories, at the intermediate stages of concrete leaching, when the pH is controlled by the dissolution of portlandite. The influence of layer nature, octahedral occupation, presence of tetrahedral Al and degree of crystallinity will be assessed by analysing the behaviour of a set of well-selected phyllosilicates and using the combined capabilities of 29Si and 27Al MAS-NMR spectroscopy, powder X-ray diffraction and SEM/EDX. The results show that the main factor affecting the stability of the clay is the octahedral occupation, so that trioctahedral phyllosilicates are much more stable than dioctahedral ones. The nature and expandability of the layer does not seem to much influence the stability of the clay, so that a 2:1 expandable phyllosilicate shows the same stability as a chemically analogous 1:1 non-expandable phyllosilicate. However other factors like the poor crystallinity of the starting material or the presence of Al in the tetrahedral sheet of trioctahedral phyllosilicates weaken the clay structure in alkaline conditions and favour the transformation towards other phases. 相似文献
19.
Residual strength after liquefaction: A rheological approach 总被引：1，自引：0，他引：1
The motion of a sphere pulled through liquefied sand of low relative density has been observed. Long triaxial specimens were prepared around a 12.7 mm-diameter sphere loaded by a wire/deadweight system. Velocities and drag forces were measured over a large range of shear strains and strain rates. Typical behavior involved a rapid drop to a non-zero minimum drag resistance followed by an increase in resistance with velocity. These results suggest that residual strength of sand after liquefaction is rate-dependent, and that the Bingham Plastic model seems a reasonable fit to the observed behavior over a large range of sliding velocities. Shear stresses calculated from the hydrodynamics of the sphere are of the same order as those inferred from field case histories. 相似文献
20.
The occurrence and the chemical compositions of ore minerals (especially the silver‐bearing minerals) and fluid inclusions of the El Zancudo mine in Colombia were investigated in order to analyze the genetic processes of the ore minerals and to examine the genesis of the deposit. The El Zancudo mine is a silver–gold deposit located in the western flank of the Central Cordillera in Antioquia Department. It consists mainly of banded ore veins hosted in greenschist and lesser disseminated ore in porphyritic rocks. The ore deposit is associated with extensive hydrothermally altered zones. The ores from the banded veins contain sphalerite, pyrite, arsenopyrite, galena, Ag‐bearing sulfosalts, Pb‐Sb sulfosalts, and minor chalcopyrite, electrum, and native silver. Electrum is included within sphalerite, pyrite, and arsenopyrite, and is also partially surrounded by pyrite, arsenopyrite, sphalerite, and tetrahedrite. Native silver is present in minor amounts as small grains in contact with Ag‐rich sulfosalts. Silver‐bearing sulfosalts are argentian tetrahedrite–freibergite solid solution, andorite, miargyrite, diaphorite, and owyheeite. Pb‐Sb sulfosalts are bournonite, jamesonite, and boulangerite. Two main crystallization stages are recognized, based on textural relations and mineral assemblages. The first‐stage assemblage includes sphalerite, pyrite, arsenopyrite, galena and electrum. The second stage is divided into two sub‐stages. The first sub‐stage commenced with the deposition and growth of sphalerite, pyrite, and arsenopyrite. These minerals are characterized by compositional growth banding, and seem to have crystallized continuously until the end of the second sub‐stage. Tetrahedrite, Pb‐Cu sulfosalts, Ag‐Sb sulfosalt, and Pb‐Ag‐Sb sulfosalts crystallized from the final part of the first sub‐stage and during the whole second sub‐stage. However, one Pb‐Ag‐Sb sulfosalt, diaphorite, was formed by a retrograde reaction between galena and miargyrite. The minimum and maximum genetic temperatures estimated from the FeS content of sphalerite coexisting with pyrite and the silver content of electrum are 300°C and 420°C, respectively. These estimated genetic temperatures are similar to, but slightly higher than the homogenization temperatures (235–350°C) of primary fluid inclusions in quartz. The presence of muscovite in the altered host rocks and gangue suggest that the pH of the hydrothermal solutions was close to neutral. Most of the sulfosalts in this deposit have previously been attributed as the products of epithermal mineralization. However, El Zancudo can be classified as a xenothermal deposit, in view of the low pressure and high temperature genetic conditions identified in the present study, based on the mineralogy of sulfosalts and the homogenization temperatures of the fluid inclusions. 相似文献